Direct backward third-harmonic generation in nanostructures

Magnetization - induced optical third - harmonic generation in Co and Fe nanostructures

Magnetization-induced optical third-harmonic generation (MTHG) is observed in magnetic nanos-tructures: Co and F e nanolayers and granular films containing Co nanoparticles. Magnetization-induced variations of the MTHG characteristics in these nanostructures exceed the typical values of linear magneto-optical Kerr effect by at least an order of magnitude: the maximum of magnetic contrast in the...

Interferometric Backward Third Harmonic Generation Microscopy for Axial Imaging with Accuracy Beyond the Diffraction Limit

A new nonlinear microscopy technique based on interference of backward-reflected third harmonic generation (I-THG) from multiple interfaces is presented. The technique is used to measure height variations or changes of a layer thickness with an accuracy of up to 5 nm. Height variations of a patterned glass surface and thickness variations of fibroblasts are visualized with the interferometric e...

Mode analysis of second-harmonic generation in plasmonic nanostructures

Using a surface integral equation approach based on the tangential Poggio–Miller–Chang–Harrington–Wu–Tsai formulation, we present a full wave analysis of the resonant modes of 3D plasmonic nanostructures. This method, combined with the evaluation of second-harmonic generation, is then used to obtain a better understanding of their nonlinear response. The second-harmonic generation associated wi...

Direct quasi-phase-matched fourth-harmonic generation.

We have theoretically demonstrated direct fourth-harmonic generation (FHG) based on a quasi-phase-matching (QPM) configuration in periodically poled lithium niobate. The wavelength dependence of period of FHG QPM gratings is calculated. Bandwidths of fundamental wavelength, temperature, and incident angle are also studied. We find a very wide bandwidth, as large as 115 nm, of fundamental wavele...

Continuous third harmonic generation in a terahertz driven modulated nanowire